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Self-nanomicellizing solid dispersion of edaravone: part II: in vivo assessment of efficacy against behavior deficits and safety in Alzheimer’s disease model

Bibliographic

Year of Publication:
2018
Contact PI Name:
Xin-Fu Zhou
Contact PI Affiliation:
School of Pharmacy and Medical Sciences, University of South Australia, Adelaide, SA , Australia
Co-Authors:
Ankit Parikh, Krishna Kathawala, Jintao Li, Chi Chen, Zhengnan Shan, Xia Cao, Yan-Jiang Wang, Sanjay Garg
Primary Reference (PubMED ID):
Funding Source:
Fujian Kangshimei Co., China
University of South Australia University President’s Scholarship
National Health and Medical Research Council of Australia
Study Goal and Principal Findings:

Background: Alzheimer's disease (AD) is a devastating neurodegenerative disorder that lacks any disease-modifying drug for the prevention and treatment. Edaravone (EDR), an approved free radical scavenger, has proven to have potential against AD by targeting multiple key pathologies including amyloid-beta (Aβ), tau phosphorylation, oxidative stress, and neuroinflammation. To enable its oral use, novel edaravone formulation (NEF) was previously developed. The aim of the present investigation was to evaluate safety and efficacy of NEF by using in vitro/in vivo disease model.

Materials and methods: In vitro therapeutic potential of NEF over EDR was studied against the cytotoxicity induced by copper metal ion, H2O2 and Aβ42 oligomer, and cellular uptake on SH-SY5Y695 amyloid-β precursor protein (APP) human neuroblastoma cell line. For in vivo safety and efficacy assessment, totally seven groups of APP/PS1 (five treatment groups, one each as a basal and sham control) and one group of C57BL/6 mice as a positive control for behavior tests were used. Three groups were orally treated for 3 months with NEF at an equivalent dose of EDR 46, 138, and 414 µmol/kg, whereas one group was supplied with each Donepezil (5.27 µM/kg) and Soluplus (amount present in NEF of 414 µmol/kg dose of EDR). Behavior tests were conducted to assess motor function (open-field), anxiety-related behavior (open-field), and cognitive function (novel objective recognition test, Y-maze, and Morris water maze). For the safety assessment, general behavior, adverse effects, and mortality were recorded during the treatment period. Moreover, biochemical, hematological, and morphological parameters were determined.

Results: Compared to EDR, NEF showed superior cellular uptake and neuroprotective effect in SH-SY5Y695 APP cell line. Furthermore, it showed nontoxicity of NEF up to 414 µM/kg dose of EDR and its potential to reverse AD-like behavior deficits of APP/PS1 mice in a dose-dependent manner.

Conclusion: Our results indicate that oral delivery of NEF holds a promise as a safe and effective therapeutic agent for AD.

Therapeutic Agent

Therapeutic Information:
Therapy Type:
Small Molecule
Therapeutic Agent:
Edaravone
Therapeutic Target:
Multi Target
Therapy Type:
Small Molecule
Therapeutic Agent:
Novel Edaravone Formulation (NEF)
Therapeutic Target:
Multi Target
Therapy Type:
Small Molecule
Therapeutic Agent:
Donepezil
Therapeutic Target:
Acetylcholinesterase
Therapeutic Notes:
To enable its oral use, novel edaravone formulation (NEF) was previously developed. The aim of the present investigation was to evaluate safety and efficacy of NEF by using in vitro/ in vivo disease model. The novel edaravone formulation (NEF) was developed, by using the strategy called self-nanomicellizing solid dispersion which is the combination of solid dispersion and nanomicelles strategies.

Animal Model

Model Information:
Species:
Mouse
Model Type:
APPxPS1
Strain/Genetic Background:
C57BL/6
Animal Model Notes:
The authors do not specify which APP/PS1 model is used in this study.

Experimental Design

Is the following information reported in the study?:
Power/Sample Size Calculation
Randomized into Groups
Blinded for Treatment
Blinded for Outcome Measures
Pharmacokinetic Measures
Pharmacodynamic Measures
Toxicology Measures
ADME Measures
Biomarkers
Dose
Formulation
Route of Delivery
Duration of Treatment
Frequency of Administration
Age of Animal at the Beginning of Treatment
Age of Animal at the End of Treatment
Sex as a Biological Variable
Study Balanced for Sex as a Biological Variable
Number of Premature Deaths
Number of Excluded Animals
Statistical Plan
Genetic Background
Inclusion/Exclusion Criteria Included
Conflict of Interest

Outcomes

Outcome Measured
Outcome Parameters
Behavioral
Morris Water Maze
Open Field Test
Y Maze
Novel Object Recognition Test (NORT)
Cell Biology
Cytotoxicity
Toxicology
Body Weight
General Behavior
Mortality
Food Intake
Water Consumption
Organ Weight
Tissue Histopathological Profile
Blood/Serum Clinical Chemistry
Physiology
Hematological Parameters
Coagulation Parameters
Serum Biochemistry